Toward bio-inspired information processing with networks of nano-scale switching elements

Unconventional computing explores multi-scale platforms connecting molecular-scale devices into networks for the development of scalable neuromorphic architectures, often based on new materials and components with new functionalities. We review some work investigating the functionalities of locally connected networks of different types of switching elements as computational substrates. In particular, we discuss reservoir computing with networks of nonlinear nanoscale components. In usual neuromorphic paradigms, the network synaptic weights are adjusted as a result of a training/learning process. In reservoir computing, the non-linear network acts as a dynamical system mixing and spreading the input signals over a large state space, and only a readout layer is trained. We illustrate the most important concepts with a few examples, featuring memristor networks with time-dependent and history dependent resistances

Interference effects in phtalocyanine controlled by H-H tautomerization: a potential two-terminal unimolecular electronic switch

We investigate the electrical transport properties of two hydrogen tautomer configurations of phthalocyanine (H2Pc) connected to cumulene and gold leads. Hydrogen tautomerization affects the electronic state of H2Pc by switching the character of molecular orbitals with the same symmetry close to the Fermi level. The near degeneracy between the HOMO and HOMO-1 leads to pronounced interference effects, causing a large change in current for the two tautomer configuratons, especially in the low-bias regime. Two types of planar junctions are considered: cumulene-H2Pc-cumulene and gold-H2Pc-gold. Both demonstrate prominent difference in molecular conductance between ON and OFF states. In addition, junctions with gold leads show pronounced negative differential resistance (NDR) at high bias voltage, as well as weak NDR at intermediate bias.Comment: 10 pages, 7 figures, accepted for publication in Physical Review

Controlling Josephson transport by manipulation of Andreev levels in ballistic mesoscopic junctions

We discuss how to control dc Josephson current by influencing the structure and nonequilibrium population of Andreev levels via external electrostatic gates, external current injection and electromagnetic radiation. In particular we will consider the "giant" Josephson current in "long" SIS tunnel junctions and the regular and anomalous nonequilibrium Josephson currents in three terminal SNS junctions. We will briefly discuss applications to the Josephson field effect transistor (JOFET) and to the newly invented Josephson interference transistor (JOINT).Comment: 10 pages, 3 figures; contribution to a special volume of Superlattices and Microstructures journal (ed. P.F. Bagwell

Multiple Andreev reflections as a transport problem in energy space

We present an approach for analyzing the dc current in voltage biased quantum superconducting junctions. By separating terms from different $n$-particle processes, we find that the $n$-particle current can be mapped on the problem of wave transport through a potential structure with $n$ barriers. We discuss the relation between resonances in such structures and the subgap structures in the current-voltage characteristics. At zero temperature we find, exactly, that only processes creating real excitations contribute to the current. Our results are valid for a general SXS-junction, where the X-region is an arbitrary non-superconducting region described by an energy-dependent transfer matrix.Comment: 11 pages, 4 figures, submitted to Superlattices and Microstructure

Resonant transport through midgap states in voltage-biased Josephson junctions of d-wave superconductors

We study theoretically the ac Josephson effect in voltage biased planar junctions of d-wave superconductors. For some orientations of the superconductors a current peak is found at finite voltage in the current-voltage characteristics. We pick out the relevant physical processes and write down an analytical formula for the current which clearly shows how the midgap state acts as a resonance and produces the peak. We present a possible explanation for the zero-bias conductance peak, recently found in experiments on grain boundary junctions of high-temperature superconductors, in terms of resonant transmission through midgap state of quasiparticles undergoing multiple Andreev reflections. We note that within our framework the zero-bias conductance peak appears in rather transparent Josephson junctions of d-wave superconductors.Comment: 10 pages, 5 figures, Submitted to a special volume of "Superlattices and Microstructures

Full Frequency Back-Action Spectrum of a Single Electron Transistor during Qubit read-out

We calculate the spectral density of voltage fluctuations in a Single Electron Transistor (SET), biased to operate in a transport mode where tunneling events are correlated due to Coulomb interaction. The whole spectrum from low frequency shot noise to quantum noise at frequencies comparable to the SET charging energy $(E_{C}/\hbar)$ is considered. We discuss the back-action during read-out of a charge qubit and conclude that single-shot read-out is possible using the Radio-Frequency SET.Comment: 4 pages, 5 figures, submitted to PR

Attosecond electron-spin dynamics in Xe 4d photoionization

The photoionization of xenon atoms in the 70-100 eV range reveals several fascinating physical phenomena such as a giant resonance induced by the dynamic rearrangement of the electron cloud after photon absorption, an anomalous branching ratio between intermediate Xe$^+$ states separated by the spin-orbit interaction and multiple Auger decay processes. These phenomena have been studied in the past, using in particular synchrotron radiation, but without access to real-time dynamics. Here, we study the dynamics of Xe 4d photoionization on its natural time scale combining attosecond interferometry and coincidence spectroscopy. A time-frequency analysis of the involved transitions allows us to identify two interfering ionization mechanisms: the broad giant dipole resonance with a fast decay time less than 50 as and a narrow resonance at threshold induced by spin-flip transitions, with much longer decay times of several hundred as. Our results provide new insight into the complex electron-spin dynamics of photo-induced phenomena

Superconducting d-wave junctions: The disappearance of the odd ac components

We study voltage-biased superconducting planar d-wave junctions for arbitrary transmission and arbitrary orientation of the order parameters of the superconductors. For a certain orientation of the superconductors the odd ac components disappear, resulting in a doubling of the Josephson frequency. We study the sensitivity of this disappearance to orientation and compare with experiments on grain boundary junctions. We also discuss the possibility of a current flow parallel to the junction.Comment: 5 pages, 3 figure

Full frequency voltage noise spectral density of a single electron transistor

We calculate the full frequency spectral density of voltage fluctuations in a Single Electron Transistor (SET), used as an electrometer biased above the Coulomb threshold so that the current through the SET is carried by sequential tunnel events. We consider both a normal state SET and a superconducting SET. The whole spectrum from low frequency telegraph noise to quantum noise at frequencies comparable to the SET charging energy $(E_{C}/\hbar)$, and high frequency Nyquist noise is described. We take the energy exchange between the SET and the measured system into account using a real-time diagrammatic Keldysh technique. The voltage fluctuations determine the back-action of the SET onto the measured system and we specifically discuss the case of superconducting charge qubit read-out and measuring the so-called Coulomb staircase of a single Cooper pair box.Comment: 14 pages, 18 figures, submitted to PR